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My friends and I donate to the Little Hats Big Hearts group as well as Children's National Medical Center in Washington DC. The link has sub-hyperlinks for each state. This group specifies red hats, but they will take any and all donations for the NICU, Newborn and Pediatric wards.
http://www.heart.org/HEARTORG/Affiliate/Little-Hats-Big-Hearts_UCM_470829_SubHomePage.jsp
http://www.heart.org/HEARTORG/Affiliate/Little-Hats-Big-Hearts_UCM_470829_SubHomePage.jsp